So why would you add to that already high risk for disaster?
Believe me, I'm rooting for you in this as I would hate to see anybody's hard work and money go in such a disastrous way. However, not a single person has sided with you in this build and a lot of very experienced fish keepers have told you it's a bad idea. I have no doubt that the casters will hold the weight but what will eventually fail is the crossmembers that run in between them. I know you used 6x6's and braced them together, and all of that, but you are talking about 4-5 tons of water/tank weight. That frame you built will eventually warp under that weight and I'm guessing it won't take very long. When that happens it will definitely cause a seem to break apart somewhere on the tank, and then you will have incredible damage to your house, not to mention whatever money you have tied up in fish in the aquarium. Think about the creaks in the second floor of a house. People are walking on boards that are anywhere between 2x6's to 2x12's depending on the building and those boards warp. I know that you are building your frame stronger than a standard floor, but you are also essentially stacking two Suburbans on top of it. I think you are taking way too much of a chance here but it's your build and your house, so I can do nothing but sit back and watch, and hope you will end up taking everyone's advice.
You are not at a point where you can't simply take the casters and leveling bolts off and just the frame by itself flat on the ground. I really hope you'll reconsider trying this but if not, I wish you the best of luck.